There are 32 Secrets of London in Assassin's Creed Syndicate. Finding all of their locations unlocks the Godlike trophy / achievement and the Aegis Outfit for Evie.
The secrets are music boxes that you must pick up. You can hear them when close enough. Use eagle vision to locate them quicker. Unlike other collectibles there isn't a map available at merchants. You can buy a map from the E-Store with microtransactions, but this costs real money.

Once all London Secrets have been found you must bring them back to Reuge's Vault. Interact with all levers in the vault and you will unlock the Aegis outfit and the Godlike trophy / achievement. You also receive 4 skill points.

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All Assassin's Creed Syndicate Trophies and Achievements:

Master Assassin
Earn every other trophy.

A Spanner in the Works
Complete Memory Sequence 1.

A Simple Plan
Complete Memory Sequence 2.

A Modern Babylon
Complete Memory Sequence 3.

A Quick and Reliable Remedy
Complete Memory Sequence 4.

The Perils of Business
Complete Memory Sequence 5.

A Run on the Bank
Complete Memory Sequence 6.

All Is Fair in Politics
Complete Memory Sequence 7.

The Joys of Freedom
Complete Memory Sequence 8.

Shall We Dance?
Complete Memory Sequence 9.

Friends at My Back
Recruit a gang of 5 allies.

The War at Home
Complete the World War I simulation.

Cerevisaphile
Sample every beer brand in London.

No Ticket
Kick fifty enemies off of trains.

Flawless Conqueror
Secure three Gang Strongholds and complete their optional constraints.

Bare-Knuckle Champion
Win three different Fight Clubs.

A Quarter-Furlong at a Time
Finish first in 3 different Street Races.

Treasure Hunter
Complete ten Raids of any type with Jacob or Evie.

Thieftaker
Bring three Bounty targets back alive.

Unqualified Success
Complete three Templar Hunts and their challenges.

Children's Aid Society
Complete five Child Liberation memories.

Guardian Angel
Successfully escort ten friendly cargo shipments.

Godlike
Unlock all of the Secrets of London.

A Broad Base
Reach Loyalty level 1 with all Associates.

Bedfellows, Strange or Otherwise
Reach maximum Loyalty with any Associate.

Needle in a Haystack
Kill five enemies from within the same haystack.

Street Sweeping
Conquer all the boroughs in London

Multitalented
Acquire ten Perks.

Keys to the City
Acquire all of the Gang Upgrades.

Artisan
Craft a Level 10 Item.

Bartitsu
Learn every Fight Skill as Jacob.

Phantom
Learn every Stealth Skill as Evie.

Wonder of the Age
Reach Level 10.

Ordinary Criminal
Complete twenty Crowd Events.

Language of Flowers
Collect all of the Pressed Flowers.

Student of History
Collect all of the Historical Posters.

A Life in Letters
Collect all of the Royal Letters.

Chimney Sweep
Synchronize every Viewpoint in London.

Mentor
Reach 100% Sync in the Main Memories

Furious
Destroy twenty vehicles by ramming them.

WHAT IS WRONG WITH YOU
Flip five vehicles by shooting their horses.

Look Out Below
Kill three enemies with a single stack of hanging barrels.

You Wouldn't Steal a Policeman's Helmet
Hijack twenty police vehicles.

Queensbury Rules
Reach combo level 40.

Whirlwind of Death
Perform fifty Multi-Finishers.

Blade in the Crowd
Assassinate fifty enemies.

Opium Scourge
Affect at least four enemies simultaneously with the Hallucinogenic Dart.

Blade from Above
Air Assassinate twenty enemies from a zipline.

Most Unsporting
Shoot fifty enemies before they shoot at you.

Without a Grudge
Destroy 5000 destructibles with your carriage

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